Megilah1: 8
אֵין בֵּין סְפָרִים לִתְפִלִּין וּמְזוּזוֹת אֶלָּא שֶׁהַסְּפָרִים נִכְתָּבִין בְּכָל לָשׁוֹן, וּתְפִלִּין וּמְזוּזוֹת אֵינָן נִכְתָּבוֹת אֶלָּא אַשּׁוּרִית. רַבָּן שִׁמְעוֹן בֶּן גַּמְלִיאֵל אוֹמֵר: אַף בַּסְּפָרִים לֹא הִתִּירוּ שֶׁיִּכָּתְבוּ אֶלָּא יְוָנִית.
There is no difference between [the laws pertaining to] Books [of Scripture] and [those pertaining to] tefillin and mezuzos except that Books [of Scripture] may be written in any language, but tefillin and mezuzos may be written only in Assyrian [script]. Rabban Shimon ben Gamliel says that even Books [of Scripture] were not authorized to be written except [in] Greek.